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The main use of methanesulfonyl chloride is the formation of methanesulfonates from alco in the presence of a non-nucleophilic base. Methanesulfonates are used as intermediates in substitution reactions, elimination reactions, reductions, and rearrangement reactions. When treated with a Lewis acid, oxime methanesulfonates will undergo a facile Beckmann rearrangement.
Methanesulfonates have been occasionally used as a protecting group for alco. It is stable to acidic conditions and is cleaved back to the alco using sodium amalgam.